Yeah, I really wanted to include Faded, I took it out last second when I realized I had inexplicably forgotten Crime Scene Part One. You really can’t go wrong with anything of theirs.
Definitely give Up In It a shot if you like the rest of their stuff. I get the sense it’s usually overlooked as the standard “noisy, before they had it figured out” album, but that’s really not the case at all. It’s overall faster and more raw than what came later, but the songwriting and emotion and tension are all there. I might even put it over 1965. (And his screaming on it is incredible.)