I voted for Deloused and Frances the Mute as I could never really get in to any of their other stuff after I left university and lost the opportunity to really spend time getting in to their other records. Loved FTM though, I've got The Widow picture disk lying around somewhere, it's a real beauty and the B-side (the title track) is brilliant.
Anyway, for a bit of wet blanket who was still feeling his way around 'alternative' music at that time they really opened up the world of weird, difficult music to me so they'll always have a special place in my heart.
As an aside, never had much luck trying to see them live, the first time (Brixton) they came on late and we had to leave after half an hour to get the train back to our squalid university town, the second time (Somerset House) they cancelled and the last time (Brixton again) I got chucked out after 20 minutes for smoking.
This is later era and as good as anything they ever did...
p.s. I hate ATDI